Barnaby Dixon is an impressive puppeteer that I first heard about probably ten years ago. If you haven't checked out some of his work, do yourself a favor and spend a few minutes there first.
In this instructional video, Barnaby explains how he uses a thermoplastic polymer - a polymer that becomes flexible when it's heated above some temperature but is rigid below that same temperature. It's a great example of the polymer's glass transition phase change. Because polymers are mixtures, they don't necessarily have definite melting temperatures as pure substances like elements or compounds do. Instead they have ranges of temperatures during which they aren't quite solid or liquid but are flexible and moldable - think of hot glass being shapeable but not liquid.
I have some of this at school. It used to be available from Educational Innovations. That's where I bought it, but they sadly don't carry it anymore. Of course, just about anything is available at Amazon if you search for pcl moldeable plastic.
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